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Aaron R. Silvis, Kayla M. Hauer, Diane A. Dickie, Charles W. Machan
An entry from the Cambridge Structural Database, the world’s repository for small molecule crystal structures. The entry contains experimental data from a crystal diffraction study. The deposited dataset for this entry is freely available from the CCDC and typically includes 3D coordinates, …
Elizabeth K. Johnson, Charles W. Machan
ABSTRACT Heterogenized molecular catalysts have been the subject of increasing interest in the context of electrochemical small molecule activation due to the possibility of active site homogeneity and tunability, which can surpass many nanostructured materials. When molecular catalysts strongly interact with carbon …
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Mary Jo McCormick, Kate G. Scheerer, Charles W. Machan
High Resolution Image Download MS PowerPoint Slide The development of transition-metal based catalysts for small-molecule activation is essential to the development of viable alternative energy sources to nonrenewable fossil fuels. Herein, the synthesis and characterization of Mn( tBu phthalocyanine)Cl ( 1Cl ) …
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Mollie C. Morrow, Charles W. Machan
I n Table 4 and Table S2, the turnover frequency (TOF) values for the intrinsic catalytic activity of Ru 3 O and NHPI derived during electrolytic oxidation of CF 3 BnOH were misreported and inconsistent with the description given in the text.The …
Mollie C. Morrow, Charles W. Machan
High Resolution Image Download MS PowerPoint Slide Increasing interest in alternative methods for fuel generation and chemical synthesis has resulted in an increased focus on the development of electrocatalysts for energy relevant small molecule transformations, such as the oxidation of methanol. Partial …
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Elizabeth K. Johnson, Daniel P. Musikanth, Christopher Webber, T. Brent Gunnoe et autres
High Resolution Image Download MS PowerPoint Slide With the increase in greenhouse gas emissions and their detrimental effect on the environment, there is a push to develop a renewable way to produce H 2, a fuel source that has nonharmful byproducts, unlike …
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Michael J. Stopper, Akachukwu D. Obi, Haleigh R. Machost, Noah D. McMillion et autres
The reaction of CAAC-CS 2 betaine ( 1; CAAC = cyclic(alkyl)(amino)carbene) and alkali metal reductants under ambient conditions yields carbene-stabilized carbon disulfide radical anions as crystalline alkali metal salts. The radicals 3–5 form multinuclear clusters featuring diverse metal sulfide and disulfide interactions, …
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Mollie C. Morrow, Charles W. Machan
RR by releasing electricity from energy-rich molecules. State-of-the-art molecular systems for the AOR are divided between single-site catalysts and co-catalytic systems with redox mediators. The AOR is contextualized as an energy relevant reaction, an overview of the area is provided, foundational improvements …
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Ephraiem S. Sarabamoun, Pramod Aryal, Jonathan M. Bietsch, Maurice Curran et autres
High Resolution Image Download MS PowerPoint Slide We contrast the switching of photoluminescence (PL) of PbS quantum dots (QDs) cross-linked with photochromic diarylethene molecules with different end groups, 4,4′-(1-cyclopentene-1,2-diyl)bis[5-methyl-2-thiophenecarboxylic acid] ( 1C ) and 4,4′-(1-cyclopentene-1,2-diyl)bis[5-methyl-2-thiophenethiocarboxylic acid] ( 2T ). Our results show …
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Emma N. Cook, Luke A. Flaxman, Amelia G. Reid, Diane A. Dickie et autres
High Resolution Image Download MS PowerPoint Slide Development of earth-abundant catalysts for the reduction of dioxygen (ORR) is essential for the development of alternative industrial processes and energy sources. Here, we report a transition metal-free dicationic organocatalyst ( Ph 2 Phen 2+ …
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Megan E. Moberg, Charles W. Machan
High Resolution Image Download MS PowerPoint Slide Conspectus Human influence on the climate system was recently summarized by the sixth Intergovernmental Panel on Climate Change (IPCC) Assessment Report, which noted that global surface temperatures have increased more rapidly in the last 50 …
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Prince Verma, Mark S. Bannon, Mara K. Kuenen, S. Shanmuga Sundara Raj et autres
The fabrication of polymer-MOF composite gels holds great potential to provide emergent properties for drug delivery, environmental remediation, and catalysis. To leverage the full potential of these composites, we investigated how the presence and chemistry of polymers impact MOF formation within the …
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