Experimental study on the permeability characteristics of reconsolidated salt: Effects of gas and confining pressure

Résumé fourni par la source

Reconsolidated salt, formed from crushed halite under compaction, is a promising buffer and sealing material for deep geological repositories of high-level radioactive waste (HLW) because of its low permeability and self-healing properties. This study investigated the gas permeability behavior of reconsolidated salt with varying porosities under different confining pressures and inlet gas pressures using nitrogen gas. Based on nuclear magnetic resonance (NMR) technology, the pore structure of reconsolidated salt specimens with different porosities was tested and imaged. The experimental results demonstrate that gas permeability decreases with increasing gas and confining pressures, with gas pressure having a more pronounced effect. The observed permeability‒pressure relationship is attributed primarily to the Klinkenberg effect, with gas slippage along pore walls enhancing the measured permeability under low-pressure conditions. Using the Klinkenberg correction, the absolute permeability values of reconsolidated salt were derived, reaching as low as 10 −19 m 2 in low-porosity samples. These values are significantly lower than the apparent gas permeability, indicating excellent sealing performance comparable to or superior to that of bentonite. A logarithmic relationship between the absolute permeability and confining pressure was established, providing a quantitative basis for permeability prediction under repository stress conditions. NMR imaging results indicate that with decreasing porosity, the connectivity between pores also gradually diminishes. Additionally, the slip factor was found to increase with increasing confining pressure, underscoring the evolving influence of pore geometry on gas transport mechanisms. Permeability of reconsolidated granular salt decreases with porosity following a power-law relationship, and the healing supports its sealing effectiveness. This study provides essential data and theoretical insights for evaluating the long-term sealing performance of reconsolidated salt in salt-based HLW repositories. • Gas pressure has a more significant effect on reconsolidated salt permeability than does confining pressure. • The Klinkenberg effect is dominant in regards to reconsolidated salt because of its microporous structure. • The absolute permeability can be two orders of magnitude lower than the gas permeability. • Reconsolidated salt has favorable sealing capacity for applications in HLW repositories.

Ce résumé expose les affirmations des auteurs. BNTIC ne l’interprète pas comme une validation indépendante des résultats.