Spin excitation continuum from degenerate states in the mixed ferro-antiferromagnetic exchange system CeMgAl 11 O 19

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In the search for unconventional magnetism, exotic quantum states are characterized by a lack of order and a broad spin excitation continuum approaching zero temperature. We study the two-dimensional triangular-lattice effective spin- 1 2 system CeMgAl 11 O 19 , which shows slight disorder but no magnetic ordering down to 100 millikelvin. Spin-wave analysis in the magnetic-field–polarized state determines the spin Hamiltonian featuring a mixed ferromagnetic-antiferromagnetic nearest-neighbor exchange interaction [ J z = −0.024(5) milli–electron volts, J ⊥ = 0.056(3) milli–electron volts]. This places the system near an exactly solvable point of the spin- 1 2 triangular-lattice XXZ model ( J z = − 1 2 J ⊥ ) with extensive ground-state degeneracy. In zero field, neutron spectroscopy reveals a prominent continuum; we show that this arises from an ensemble average of spin-wave spectra across the degenerate ground-state manifold. This demonstrates that the role of weak quenched disorder can be quantitatively constrained: It inhibits unique ground-state selection and stabilizes a local distribution within the degenerate manifold, yielding continuum-like spectra that necessitate a critical reevaluation of the experimental signatures of exotic quantum states.

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