Mimicking Enzymatic Proton Channeling Enables Near‐Unity Selective Ammonia Electrosynthesis Beyond Neutral Limits
Zhihao Wang, Jiaxin Yu, Lin He, Xu Zhang et autres
ABSTRACT Fragmented hydrogen‐bond networks relegate proton transport to sluggish diffusion, leading to mismatched proton supply that compromises catalytic efficiency and selectivity, thereby necessitating strategies to enhance water‐network ordering. Inspired by the proton channel mechanism in enzymatic catalysis, this work anchors silicotungstate (SiW …
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Angewandte Chemie