Photoinduced Enhancement of Chemical Shift Sensitivity to Local Vibrations
Ana Martinez Gutierrez, Oliver Alexander, Pablo Estévez Alonso, L. Paoloni et autres
The advent of novel free-electron laser sources enabling time-resolved X-ray photoelectron spectroscopy (tr-XPS) provides a unique opportunity to monitor local chemical environments in real time by measuring sub-eV shifts in core-electron binding energies. These shifts reflect the interplay between electronic excitation and …
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Journal of the American Chemical Society